%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%% OIO %%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%%% Version 2.0 OIO_0.35nm_2005_07_01_ps (wavelength calibration improved) (previous: OIO_0.35nm_2005_05_25_ps) Recorded and analysed by: Peter Spietz, Juan Carlos Gómez Martín and John P. Burrows The Institute of Environmental Physics and Remote Sensing University of Bremen 28334 Bremen PO-Box 330440 spietz@iup.physik.uni-bremen.de ---------------------------------------------------------------------- Experiment type: - Xenon flash photolysis of mixtures of I2+O3 in bath gases O2 and N2. - Flow mode - Analysis light source: Xenon arc lamp. - Detection system: - Grating spectrometer Acton Research Company SP500, 500mm focal length, grating 1200 grooves/mm. - CCD camera Roper Scientific, 1024 x 1024 pixels, 26µm x 26µm pixel size, operated in time resolved mode. - linear dispersion 0.036nm / pixel - Slit width 240 µm, Field of View filled => - Resolution: 0.35 nm FWHM (at 546.074 nm) - Reaction vessel: Quarz, 120 cm, multi path optics (White type), mirrors: Al + MgF2, path length: 990.5cm ---------------------------------------------------------------------- T=298k P=30mbar ---------------------------------------------------------------------- Analysis: -IO* and I2 background corrected by multivariate multiple linear regression -one spectral window:[532-568nm] ---------------------------------------------------------------------- Vertical axis: Absolute scaling obtained by an iodine conservation approach sigma(549.4nm vac)=(1.3±0.3)E-17cm2 at 0.35 nm FWHM ---------------------------------------------------------------------- Horizontal axis: -Calibrated against Platinum-Chromium/Neon line source measurement (wavelength in air). Residuals below 0.03 nm. -Transferred to vaccuum wavelength by Edlen's formula (see Morton (1991) ApJS, 77, 119) ---------------------------------------------------------------------- lambda_air: air wavelength (nm) lambda_vac: vacuum wavelength (nm) wavenumber: vacuum wavenumber (cm-1) rel: relative spectrum (optical density) (dimensionless) error_rel: error relative spectrum (dimensionless) abs: Absolutely scaled spectrum (cm2) error_abs:error absolute spectrum (cm2) relative_error_abs: relative error of the absolutely scaled spectrum ---------------------------------------------------------------------- ---------------------------------------------------------------------- Data: lambda_air lambda_vac wavenumber rel error_rel abs error_abs relative_error_abs ------------------------------------------------------------------------------------------ 532.81251 532.96073 18763.10858 0.01262 7.30498E-4 5.59001E-18 1.33541E-18 0.23889 532.84712 532.99535 18761.88987 0.0122 7.66216E-4 5.40225E-18 1.29728E-18 0.24014 532.88173 533.02997 18760.67133 0.01152 7.83306E-4 5.10263E-18 1.2325E-18 0.24154 532.91634 533.06459 18759.45294 0.01133 7.53973E-4 5.01555E-18 1.20949E-18 0.24115 532.95095 533.0992 18758.23471 0.01109 7.59357E-4 4.90871E-18 1.18638E-18 0.24169 532.98556 533.13382 18757.01663 0.01151 7.50263E-4 5.0985E-18 1.22754E-18 0.24076 533.02017 533.16844 18755.79872 0.01142 7.31136E-4 5.0554E-18 1.21564E-18 0.24046 533.05478 533.20306 18754.58096 0.01104 7.28021E-4 4.88892E-18 1.17811E-18 0.24098 533.08939 533.23768 18753.36337 0.01083 7.08356E-4 4.79732E-18 1.15531E-18 0.24082 533.124 533.2723 18752.14593 0.01048 7.26734E-4 4.6425E-18 1.12312E-18 0.24192 533.15861 533.30692 18750.92864 0.01072 7.28719E-4 4.74486E-18 1.14612E-18 0.24155 533.19322 533.34154 18749.71152 0.0103 7.04123E-4 4.56109E-18 1.10218E-18 0.24165 533.22783 533.37616 18748.49455 0.01033 7.03187E-4 4.57506E-18 1.10517E-18 0.24156 533.26245 533.41079 18747.27739 0.01006 6.74257E-4 4.45433E-18 1.07472E-18 0.24128 533.29706 533.44541 18746.06074 0.01008 7.10587E-4 4.46319E-18 1.08127E-18 0.24226 533.33167 533.48003 18744.84425 0.00957 6.75945E-4 4.23645E-18 1.02652E-18 0.24231 533.36628 533.51465 18743.62792 0.00939 6.86589E-4 4.15974E-18 1.01094E-18 0.24303 533.40089 533.54926 18742.41174 0.00926 6.69376E-4 4.09953E-18 9.95342E-19 0.24279 533.4355 533.58388 18741.19572 0.00943 6.41146E-4 4.17587E-18 1.00866E-18 0.24154 533.47011 533.6185 18739.97986 0.00951 6.56629E-4 4.21219E-18 1.01867E-18 0.24184 533.50472 533.65312 18738.76416 0.00975 6.68571E-4 4.31952E-18 1.04403E-18 0.2417 533.53933 533.68774 18737.54861 0.00928 6.69973E-4 4.10957E-18 9.97643E-19 0.24276 533.57394 533.72236 18736.33323 0.00946 6.59252E-4 4.18838E-18 1.01372E-18 0.24203 533.60855 533.75698 18735.118 0.00912 6.62752E-4 4.0369E-18 9.80611E-19 0.24291 533.64316 533.7916 18733.90293 0.0093 6.55806E-4 4.11637E-18 9.97302E-19 0.24228 533.67777 533.82622 18732.68801 0.00883 6.55837E-4 3.90962E-18 9.51566E-19 0.24339 533.71238 533.86084 18731.47325 0.00897 6.18685E-4 3.97322E-18 9.60795E-19 0.24182 533.74699 533.89546 18730.25865 0.00897 6.39802E-4 3.97158E-18 9.63138E-19 0.24251 533.7816 533.93008 18729.04421 0.00888 6.42676E-4 3.93244E-18 9.5485E-19 0.24281 533.81621 533.9647 18727.82993 0.00912 6.53117E-4 4.03853E-18 9.79704E-19 0.24259 533.85082 533.99931 18726.6158 0.0088 6.43655E-4 3.89697E-18 9.47136E-19 0.24304 533.88543 534.03393 18725.40183 0.00885 6.37249E-4 3.91691E-18 9.50699E-19 0.24272 533.92004 534.06855 18724.18802 0.00889 6.35916E-4 3.93685E-18 9.5494E-19 0.24256 533.95465 534.10317 18722.97436 0.00871 6.14473E-4 3.85711E-18 9.34487E-19 0.24228 533.98926 534.13779 18721.76087 0.00869 6.12451E-4 3.8469E-18 9.31961E-19 0.24226 534.02388 534.17242 18720.54717 0.00851 6.36249E-4 3.76719E-18 9.17483E-19 0.24355 534.05849 534.20704 18719.33399 0.00799 6.22533E-4 3.5371E-18 8.64929E-19 0.24453 534.0931 534.24166 18718.12097 0.00818 6.11132E-4 3.62419E-18 8.82524E-19 0.24351 534.12771 534.27628 18716.9081 0.00829 6.16295E-4 3.66924E-18 8.93165E-19 0.24342 534.16232 534.3109 18715.69539 0.00819 6.13134E-4 3.62489E-18 8.82951E-19 0.24358 534.19693 534.34552 18714.48283 0.00791 7.43217E-4 3.50294E-18 8.76071E-19 0.2501 534.23154 534.38014 18713.27043 0.0079 6.30236E-4 3.49888E-18 8.57641E-19 0.24512 534.26615 534.41476 18712.05819 0.00825 6.841E-4 3.65309E-18 8.99266E-19 0.24617 534.30076 534.44937 18710.84611 0.00767 6.06742E-4 3.39655E-18 8.31831E-19 0.2449 534.33537 534.48399 18709.63418 0.00719 6.29052E-4 3.18458E-18 7.88928E-19 0.24773 534.36998 534.51861 18708.42242 0.00769 6.21713E-4 3.4033E-18 8.35474E-19 0.24549 534.40459 534.55323 18707.2108 0.00737 6.25894E-4 3.26561E-18 8.06045E-19 0.24683 534.4392 534.58785 18705.99935 0.00759 6.23768E-4 3.35934E-18 8.26165E-19 0.24593 534.47381 534.62247 18704.78805 0.00745 6.23957E-4 3.29989E-18 8.13218E-19 0.24644 534.50842 534.65709 18703.57691 0.0077 6.22875E-4 3.41157E-18 8.37452E-19 0.24547 534.54303 534.69171 18702.36592 0.00715 6.1905E-4 3.16516E-18 7.83158E-19 0.24743 534.57764 534.72633 18701.1551 0.00693 6.31127E-4 3.06691E-18 7.63808E-19 0.24905 534.61225 534.76095 18699.94442 0.00708 6.70214E-4 3.1342E-18 7.84725E-19 0.25037 534.64686 534.79557 18698.73391 0.00695 6.89666E-4 3.07971E-18 7.76395E-19 0.2521 534.68147 534.83019 18697.52355 0.00661 6.76946E-4 2.92555E-18 7.41382E-19 0.25342 534.71608 534.86481 18696.31335 0.00639 7.05936E-4 2.82863E-18 7.26324E-19 0.25678 534.75069 534.89942 18695.10331 0.00605 7.30594E-4 2.6806E-18 7.00486E-19 0.26132 534.78531 534.93405 18693.89307 0.00551 7.71141E-4 2.43906E-18 6.60446E-19 0.27078 534.81992 534.96867 18692.68334 0.00529 8.00794E-4 2.34264E-18 6.48507E-19 0.27683 534.85453 535.00329 18691.47377 0.00544 8.00285E-4 2.40831E-18 6.61183E-19 0.27454 534.88914 535.03791 18690.26435 0.00522 7.96015E-4 2.30932E-18 6.40888E-19 0.27752 534.92375 535.07253 18689.05509 0.00513 7.55572E-4 2.27255E-18 6.24005E-19 0.27458 534.95836 535.10715 18687.84598 0.0053 7.46704E-4 2.34479E-18 6.36152E-19 0.2713 534.99297 535.14177 18686.63703 0.00521 7.39623E-4 2.30763E-18 6.27168E-19 0.27178 535.02758 535.17639 18685.42824 0.00526 7.24044E-4 2.32918E-18 6.27881E-19 0.26957 535.06219 535.21101 18684.2196 0.005 7.16497E-4 2.2139E-18 6.03298E-19 0.2725 535.0968 535.24563 18683.01112 0.0047 7.20006E-4 2.0801E-18 5.78006E-19 0.27787 535.13141 535.28025 18681.8028 0.00486 7.38475E-4 2.15195E-18 5.96413E-19 0.27715 535.16602 535.31487 18680.59463 0.00479 7.25361E-4 2.12147E-18 5.87322E-19 0.27685 535.20063 535.34948 18679.38662 0.00483 6.8531E-4 2.13948E-18 5.81371E-19 0.27173 535.23524 535.3841 18678.17877 0.00475 7.02756E-4 2.1022E-18 5.78139E-19 0.27502 535.26985 535.41872 18676.97107 0.00525 6.94598E-4 2.32366E-18 6.20213E-19 0.26691 535.30446 535.45334 18675.76353 0.00482 6.56839E-4 2.13627E-18 5.74249E-19 0.26881 535.33907 535.48796 18674.55614 0.00519 6.6579E-4 2.29615E-18 6.08401E-19 0.26497 535.37368 535.52258 18673.34891 0.00474 6.56461E-4 2.09903E-18 5.66738E-19 0.27 535.40829 535.5572 18672.14184 0.00501 6.40675E-4 2.21881E-18 5.87334E-19 0.26471 535.4429 535.59182 18670.93492 0.00483 6.55877E-4 2.13917E-18 5.74614E-19 0.26862 535.47751 535.62644 18669.72816 0.005 6.60604E-4 2.21421E-18 5.9072E-19 0.26679 535.51212 535.66106 18668.52156 0.0047 6.46104E-4 2.08028E-18 5.60657E-19 0.26951 535.54673 535.69568 18667.31511 0.00504 6.62008E-4 2.23268E-18 5.9475E-19 0.26638 535.58135 535.73031 18666.10846 0.00522 6.78146E-4 2.31331E-18 6.14538E-19 0.26565 535.61596 535.76493 18664.90233 0.00494 6.31497E-4 2.18916E-18 5.79352E-19 0.26465 535.65057 535.79954 18663.69634 0.00559 6.73762E-4 2.47406E-18 6.46404E-19 0.26127 535.68518 535.83416 18662.49052 0.00523 6.27846E-4 2.31794E-18 6.0492E-19 0.26097 535.71979 535.86878 18661.28485 0.0053 6.42097E-4 2.34735E-18 6.1388E-19 0.26152 535.7544 535.9034 18660.07933 0.00567 6.21887E-4 2.51018E-18 6.43686E-19 0.25643 535.78901 535.93802 18658.87397 0.00594 6.58986E-4 2.63119E-18 6.7607E-19 0.25694 535.82362 535.97264 18657.66877 0.00632 6.42634E-4 2.79651E-18 7.07885E-19 0.25313 535.85823 536.00726 18656.46372 0.00688 6.65816E-4 3.04695E-18 7.65291E-19 0.25117 535.89284 536.04188 18655.25883 0.00648 6.16706E-4 2.86957E-18 7.18985E-19 0.25055 535.92745 536.0765 18654.0541 0.00766 6.40702E-4 3.39219E-18 8.35858E-19 0.24641 535.96206 536.11112 18652.84952 0.00776 6.3501E-4 3.43681E-18 8.44752E-19 0.2458 535.99667 536.14574 18651.64509 0.00816 6.27594E-4 3.61296E-18 8.82316E-19 0.24421 536.03128 536.18036 18650.44082 0.0093 6.09265E-4 4.11903E-18 9.92091E-19 0.24086 536.06589 536.21498 18649.23671 0.00968 6.2871E-4 4.28613E-18 1.03171E-18 0.24071 536.1005 536.24959 18648.03275 0.00966 6.18899E-4 4.27631E-18 1.02835E-18 0.24048 536.13511 536.28421 18646.82895 0.01021 6.11113E-4 4.52082E-18 1.08221E-18 0.23938 536.16972 536.31883 18645.6253 0.01102 6.43178E-4 4.87959E-18 1.16629E-18 0.23901 536.20433 536.35345 18644.42181 0.01134 6.12438E-4 5.01943E-18 1.19459E-18 0.23799 536.23894 536.38807 18643.21847 0.01224 6.20088E-4 5.41851E-18 1.28556E-18 0.23725 536.27355 536.42269 18642.01529 0.01239 6.29218E-4 5.4872E-18 1.30198E-18 0.23728 536.30816 536.45731 18640.81226 0.01262 6.17464E-4 5.5875E-18 1.32361E-18 0.23689 536.34278 536.49194 18639.60904 0.01271 6.35204E-4 5.62615E-18 1.33401E-18 0.23711 536.37739 536.52656 18638.40633 0.01326 6.25241E-4 5.87035E-18 1.3885E-18 0.23653 536.412 536.56118 18637.20377 0.01303 6.1399E-4 5.76886E-18 1.36446E-18 0.23652 536.44661 536.5958 18636.00136 0.01334 6.07946E-4 5.90493E-18 1.39486E-18 0.23622 536.48122 536.63042 18634.79911 0.01313 6.08469E-4 5.81351E-18 1.37412E-18 0.23637 536.51583 536.66504 18633.59702 0.01383 6.28545E-4 6.12541E-18 1.44677E-18 0.23619 536.55044 536.69965 18632.39508 0.01374 5.84251E-4 6.08457E-18 1.43381E-18 0.23565 536.58505 536.73427 18631.19329 0.01351 6.26425E-4 5.98426E-18 1.41449E-18 0.23637 536.61966 536.76889 18629.99166 0.01369 6.43028E-4 6.06234E-18 1.43368E-18 0.23649 536.65427 536.80351 18628.79019 0.01375 6.31642E-4 6.0895E-18 1.43886E-18 0.23629 536.68888 536.83813 18627.58887 0.01343 6.49704E-4 5.94804E-18 1.40833E-18 0.23677 536.72349 536.87275 18626.3877 0.01341 6.53231E-4 5.93719E-18 1.40619E-18 0.23684 536.7581 536.90737 18625.18669 0.01301 6.6404E-4 5.76246E-18 1.3676E-18 0.23733 536.79271 536.94199 18623.98583 0.01288 7.24332E-4 5.70543E-18 1.36074E-18 0.2385 536.82732 536.97661 18622.78513 0.01308 7.59654E-4 5.79282E-18 1.38415E-18 0.23894 536.86193 537.01123 18621.58459 0.01209 7.81661E-4 5.35499E-18 1.28853E-18 0.24062 536.89654 537.04585 18620.3842 0.01206 7.76234E-4 5.34236E-18 1.28507E-18 0.24054 536.93115 537.08047 18619.18396 0.01251 7.68871E-4 5.53987E-18 1.3284E-18 0.23979 536.96576 537.11509 18617.98388 0.01236 7.702E-4 5.4726E-18 1.31348E-18 0.24001 537.00037 537.1497 18616.78395 0.01198 7.63397E-4 5.30454E-18 1.2751E-18 0.24038 537.03498 537.18432 18615.58418 0.01214 7.53767E-4 5.37452E-18 1.28964E-18 0.23995 537.06959 537.21894 18614.38456 0.01196 7.31805E-4 5.29553E-18 1.26945E-18 0.23972 537.10421 537.25357 18613.18475 0.01226 7.2737E-4 5.42987E-18 1.29909E-18 0.23925 537.13882 537.28819 18611.98545 0.01191 7.29106E-4 5.273E-18 1.2641E-18 0.23973 537.17343 537.32281 18610.78629 0.01175 7.06422E-4 5.20338E-18 1.24594E-18 0.23945 537.20804 537.35743 18609.58729 0.01114 7.18403E-4 4.93121E-18 1.1864E-18 0.24059 537.24265 537.39205 18608.38845 0.01137 6.81747E-4 5.03365E-18 1.20512E-18 0.23941 537.27726 537.42667 18607.18976 0.01157 7.09179E-4 5.1219E-18 1.22798E-18 0.23975 537.31187 537.46129 18605.99122 0.01113 7.01306E-4 4.92738E-18 1.18353E-18 0.24019 537.34648 537.49591 18604.79284 0.01108 6.98943E-4 4.90693E-18 1.17868E-18 0.24021 537.38109 537.53053 18603.59461 0.0109 6.75226E-4 4.82543E-18 1.15771E-18 0.23992 537.4157 537.56515 18602.39654 0.01088 6.96412E-4 4.81867E-18 1.15866E-18 0.24045 537.45031 537.59976 18601.19862 0.01064 6.73751E-4 4.71056E-18 1.13184E-18 0.24028 537.48492 537.63438 18600.00086 0.0105 6.92501E-4 4.6515E-18 1.12088E-18 0.24097 537.51953 537.669 18598.80325 0.01011 6.59053E-4 4.4782E-18 1.0782E-18 0.24077 537.55414 537.70362 18597.60579 0.01046 6.56935E-4 4.62977E-18 1.11181E-18 0.24014 537.58875 537.73824 18596.40849 0.01031 6.74155E-4 4.56365E-18 1.09907E-18 0.24083 537.62336 537.77286 18595.21134 0.00994 6.78672E-4 4.40201E-18 1.06363E-18 0.24162 537.65797 537.80748 18594.01435 0.01057 6.67513E-4 4.68136E-18 1.12458E-18 0.24023 537.69258 537.8421 18592.81751 0.01004 6.77981E-4 4.4451E-18 1.07313E-18 0.24142 537.72719 537.87672 18591.62082 0.01023 6.67074E-4 4.53086E-18 1.09091E-18 0.24077 537.7618 537.91134 18590.42429 0.0103 6.76049E-4 4.56212E-18 1.09896E-18 0.24089 537.79641 537.94596 18589.22792 0.01036 6.60748E-4 4.589E-18 1.10314E-18 0.24039 537.83102 537.98058 18588.03169 0.01072 6.26918E-4 4.74909E-18 1.13521E-18 0.23904 537.86564 538.01521 18586.83528 0.01024 6.6423E-4 4.53489E-18 1.09147E-18 0.24068 537.90025 538.04982 18585.63936 0.01023 6.70128E-4 4.53208E-18 1.09155E-18 0.24085 537.93486 538.08444 18584.4436 0.01027 6.51918E-4 4.54573E-18 1.09244E-18 0.24032 537.96947 538.11906 18583.24799 0.01068 6.52403E-4 4.72996E-18 1.13373E-18 0.23969 538.00408 538.15368 18582.05254 0.01079 6.52135E-4 4.77644E-18 1.14412E-18 0.23953 538.03869 538.1883 18580.85724 0.01055 6.20587E-4 4.67126E-18 1.11703E-18 0.23913 538.0733 538.22292 18579.6621 0.01075 6.09647E-4 4.7607E-18 1.13597E-18 0.23861 538.10791 538.25754 18578.4671 0.01102 6.33974E-4 4.88016E-18 1.16543E-18 0.23881 538.14252 538.29216 18577.27226 0.01145 6.41664E-4 5.07108E-18 1.20923E-18 0.23846 538.17713 538.32678 18576.07758 0.01087 6.44751E-4 4.81389E-18 1.15171E-18 0.23925 538.21174 538.3614 18574.88305 0.01096 6.29355E-4 4.85104E-18 1.15839E-18 0.23879 538.24635 538.39602 18573.68867 0.01098 6.33434E-4 4.86406E-18 1.16175E-18 0.23884 538.28096 538.43064 18572.49445 0.01067 6.29937E-4 4.72582E-18 1.13031E-18 0.23918 538.31557 538.46526 18571.30038 0.011 6.41828E-4 4.87088E-18 1.16419E-18 0.23901 538.35018 538.49987 18570.10646 0.01062 6.31466E-4 4.70164E-18 1.12504E-18 0.23929 538.38479 538.53449 18568.91269 0.01042 6.16068E-4 4.61586E-18 1.10409E-18 0.23919 538.4194 538.56911 18567.71908 0.01086 6.31091E-4 4.81059E-18 1.14948E-18 0.23895 538.45401 538.60373 18566.52563 0.01035 6.07491E-4 4.58382E-18 1.09596E-18 0.23909 538.48862 538.63835 18565.33232 0.01097 6.24282E-4 4.85801E-18 1.15942E-18 0.23866 538.52323 538.67297 18564.13917 0.01035 6.17501E-4 4.58177E-18 1.09659E-18 0.23934 538.55784 538.70759 18562.94618 0.01064 6.2984E-4 4.71298E-18 1.12741E-18 0.23921 538.59245 538.74221 18561.75333 0.01038 6.06875E-4 4.59459E-18 1.09831E-18 0.23904 538.62706 538.77683 18560.56065 0.00996 6.3809E-4 4.40973E-18 1.06042E-18 0.24047 538.66168 538.81146 18559.36776 0.01051 6.0817E-4 4.65565E-18 1.11218E-18 0.23889 538.69629 538.84608 18558.17538 0.01004 6.20928E-4 4.44752E-18 1.06688E-18 0.23988 538.7309 538.8807 18556.98315 0.0099 6.17013E-4 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