SFIT4 emission mode

General

As has been shown elsewhere (Rathke et.al. 2000, ), FTIR spectrometers can be used to record thermal emission from the atmosphere. This may be used to record amounts of trace gases in the polar winter (Mariani et.el. 2013), to evaluate different cloud properties (Rathke et.al. 2000). Taquet (2017) used sfit4 in emission mode to retrieve gas contents in a volcanic plume. Most recently a FTIR in emission mode has been used on a shipcruise in the Arctic as part of the AC3 coordinated project.

Description of radiative transfer

The emission modul of SFIT4 calculates the full radiative transfer. Please see the following scheme for an easy explanation. Basically every layer is both an absorber and emitter, as described by Kirchhoff's law. To calculate the spectrum seen at the ground (or any other place) one has to calculate the sum of the emission of each layer m minus the absorption on the way from layer m to the observer. The result is a spectrum where the lines point upward.

Example of an emission spectrum

One can clearly see the effect of an absorbing layer. It is reducing the emission coming from beyond the layer and adding a continuum on it. For the Jacobian of the spectrum is calculated using the semianlytic calculation of the Jacobian . This has the advantage, that the spectrum and the Jacobian are calculated in n steps. n is the number of layer, whereas a more tradiational approach by using a perturbation of the state of each layer would require n**2 calculations.

Modellation of absorbing layers in the atmosphere.

SFIT4 offeres several possibilites to model atmospheric layers in the atmsophere.
The continuums model I models an absorption which is proportional to the pressure, i.e. strongest on the ground and getting less in higher altitude. The absorption layer may be modelled as an polynomial. This model can be used to account for unknown absorption, e.g. a continuum of a particula gas, but is not able to draw any interference about the nature or shape of this absorption.
The continuums model II models one layer of an absorber in a specified altitude only. This can be used to model optically thin clouds. If the atmosphere is overcast with thick clouds, the cloud bottom servers as an balckbody at the temperature of its altitude. SFIT4 can to date only retrieve the optical thinckness of the cloud. Future projects are several other parameters, which is topic of the sub-projects B06 in AC3. The use of the continuum to retrieve cloud properties has been described by Rathke et al. 2000

Getting the software

SFIT4 is free to use for everybody and is also a standard retrieval software used in the NDACC network . The official version is freely available without restriction. But the part I am working on is a preliminary version and subject to frequent changes and bug fixes. Because I would like to keep track of the people using this particular version, I distribute the software only on request. I also ask you not to distribute it further, but to refer interested users to me. So if you intend to use it write an email to mathias(dot)palm(at)uni(minus)bremen(dot)de. Especially I ask you not to publish results using this software without my explicit consent.

References

C. Rathke and J. Fischer, Retrieval of Cloud Microphysical Properties from Thermal Infrared Observations by a Fast Iterative Radiance Fitting Method, Journal Of Atmospheric And Oceanic Technology, Volume 17, 2000